TMSOTf Electrolyte Additive

Stable Cycling for High-Voltage Li Metal

A trimethylsilyl trifluoromethanesulfonate additive that builds stable LiF- and Li₂SOₓ-rich interphases on both cathode and lithium metal anode, enabling stable cycling of Li||NCM622 batteries at 4.6 V.

Jiaxin, Jing · Bai, Yu · Li, Xin · Tao, Ren · 73821677 · Sun, Kening

Energy Storage Materials 2025

Advantages

Stable cycling at high cut-off voltage of 4.6 V

Interphases enriched with LiF and Li₂SOₓ (x = 0, 3, 4)

Scavenges HF in electrolyte to inhibit corrosion